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Mathilda Simmons is a nun in a cult, which Ash Landers claims to have the Book of Doomsday.
Mathilda possesses big green eyes and long auburn hair, as well as pale skin. As a nun, she wears a black and white-colored robe, and a black hood with the symbol identical to that of the one seen upon Ciel Phantomhive's lower back.
Mathilda works as a nun who is brainwashed by a cult, thinking that everyone must be pure. When Ash Landers claims that her abbey has the Book of Doomsday, Sebastian Michaelis sets out to seduce her and make her 'impure' in order to extract more information.
Her Cinematic Record book is used by Undertaker to transport Sebastian, Grell Sutcliff and William T. Spears to the monastery. The three fight Angela upon getting there; Sebastian claims he has marked her and is unharmed by the angelic attacks.
- Mathilda is briefly seen in the the first OVA, post-credits.